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  • Synthesis and evaluation of diphenylphosphinic amides and diphenylphosphine oxides as inhibitors of Kv1.5.

Synthesis and evaluation of diphenylphosphinic amides and diphenylphosphine oxides as inhibitors of Kv1.5.

Bioorganic & medicinal chemistry letters (2012-12-25)
Roine I Olsson, Ingemar Jacobson, Jonas Boström, Tomas Fex, Annika Björe, Christina Olsson, Johan Sundell, Ulrik Gran, Anna Öhrn, Andreas Nordin, Jonna Gyll, Maria Thorstensson, Ahlke Hayen, Karolina Aplander, Olle Hidestål, Fanyi Jiang, Gunilla Linhardt, Elin Forsström, Teresa Collins, Monika Sundqvist, Emma Lindhardt, Annika Åstrand, Boel Löfberg
ABSTRACT

Diphenylphosphinic amides and diphenylphosphine oxides have been synthesized and tested as inhibitors of the Kv1.5 potassium ion channel as a possible treatment for atrial fibrillation. In vitro structure-activity relationships are discussed and several compounds with Kv1.5 IC(50) values of <0.5 μM were discovered. Selectivity over the ventricular IKs current was monitored and selective compounds were found. Results from a rabbit PD-model are included.

MATERIALS
Product Number
Brand
Product Description

Sigma-Aldrich
Biphenyl, ≥99%
Supelco
Biphenyl solution, certified reference material, 2000 μg/mL in methanol
Supelco
Biphenyl, PESTANAL®, analytical standard
Sigma-Aldrich
Biphenyl, ReagentPlus®, 99.5%